Dielectric loss and defect mode of SrTiO3 thin films under direct-current bias

The dielectric behavior of SrTiO3 thin films prepared by the pulsed-laser deposition technique on SrTiO3 single-crystal substrates is studied under dc electric field. A high dielectric constant maximum «max(;2280) and a low-loss tan d (;0.001) are obtained. Compared with the observation in SrTiO3 single crystals, an additional dielectric loss peak with frequency dispersion is observed around 150 K ~at 1 kHz!. With increasing dc bias, the peak is suppressed and finally disappears at ;350 kV/cm; however, the temperature at which the peak occurs is independent of electric field. The possible physical mechanism of the peak is briefly discussed. © 2001 American Institute of Physics. @DOI: 10.1063/1.1367299#